Frequency stable and low phase noise THz synthesis for precision spectroscopy

Léo Djevahirdjian, Loïc Lechevallier, Marie-Aline Martin-Drumel, Olivier Pirali, Guillaume Ducournau, Rédha Kassi, Samir Kassi
Nature Communications
14,
7162
(2023)
First page of Djevahirdjian et al. 2023, Nature Communications
Djevahirdjian et al. (2023)
Nature Communications 14, 7162

Research overview

Researchers at the Université Grenoble Alpes (LIPhy), the Institut des Sciences Moléculaires d’Orsay and IEMN Lille built a continuously tunable terahertz source from 0.1 to 1.4 THz with Hz-level linewidth and very low phase noise. Two commercial telecom DFB lasers are locked by optical feedback to a single highly stable V-shaped cavity, and their beat note is converted to THz by photomixing. The phase noise was measured up to 1.2 THz, and the long-term drift is about 0.15 mHz/s. To show what the source can do, the team recorded low-pressure methanol and water absorption lines up to 1.4 THz. They also resolved the hyperfine structure of the 556.9 GHz water line by saturation (Lamb-dip) spectroscopy, with features only 10 kHz wide. In the sub-Doppler setup, a wire-grid polarizer separated the returning beam from the incoming one in a double-pass absorption cell.

Key findings

  • Two telecom DFB lasers locked by optical feedback to one V-shaped cavity give a continuously tunable THz source from 0.1 to 1.4 THz by photomixing.
  • Hz-level linewidth was demonstrated by phase-noise measurements up to 1.2 THz, with a long-term drift of about 0.15 mHz/s.
  • Low-pressure methanol and water absorption lines were recorded up to 1.4 THz, with sub-kHz frequency accuracy referenced to an optical frequency comb.
  • Saturation spectroscopy resolved the hyperfine structure of the 556.9 GHz water line, with Lamb dips about 10 kHz wide.
  • A roof-top mirror rotated the returning beam’s polarization by 90°, and a polarization grid separated it from the incident beam in the double-pass cell.
Djevahirdjian et al.,
2023

Publication details

Journal

Nature Communications

Volume

14

Issue

Article

7162

Published

2023

Research area

Spectroscopy and Molecular Physics

Application

Ultra-high-resolution THz molecular spectroscopy

Institution

Université Grenoble Alpes, CNRS, LIPhy